Lasers for Metrology – Measuring Properties and Testing Theories at the Limits

The importance of time measurement for mankind is not an invention of the last centuries. Ancient calendars, like Stonehenge might be one, exist since thousands of years.
The importance of time measurement for mankind is not an invention of the last centuries. Ancient calendars, like Stonehenge might be one, exist since thousands of years.
  • Time & frequency 
  • Fundamental constants and tests of fundamental theories
  • Atom interferometry, rotation & acceleration
  • Laser-based trace gas analysis (ATTA, RIMS)
  • TOPTICA’s added value

Metrology is one of the oldest branches of science, applied already thousands of years before Christ. People observed the movement of the sun and the moon to measure time. This allowed them to determine the best periods for seeding and for winter preparation. Time was so important that mayn cultures erected marvelous buildings, religious sites – like potentially Stonehenge – to honor their gods, the sun and the moon. Later, it became also obvious that precise measurement of time is needed for proper navigation, leading to more and more precise clocks. 

Today, high precision frequency measurements on cold atoms or trapped ions give time and length standards and are improving the resolution of global positioning systems. They are used to determine fundamental constants, like the fine structure constant α or the Rydberg constant, and to test basic principles in physics, like the time independence of fundamental constants. 

Atom interferometers are used to measure gravity (gravimeters) or rotations (gyroscopes) with highest accuracy. They can be used for earth quake and volcano eruption research, to find natural resources or hidden subterrestrial structures and to test earth tide models, the weak equivalence principle and general relativity.  

Spectroscopic gas analysis is used to monitor gas flow. Sophisticated laser based methods for trace gas analysis and isotope ratio determination were developed to measure pollution, the age of ancient material or ground water and to detect plutonium production.
 

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Time & frequency measurement is since 1967 referred to a cesium atom standard. One second is defined as the time needed for 9,192,631,770 oscillations of the 133Cs atom's resonance frequency for its m=0 to m=0 transition between the two hyperfine levels of the electronic ground state. Consequently, the measurement is performed at microwave frequencies in a spectroscopic way that was developed by Rabi (Nobel Prize in Physics in 1944) and refined by Ramsey (Nobel Prize in Physics in 1989). First Cs atomic clocks were based on atomic beams. Newer realizations, so-called fountain clocks, use atomic fountains to increase the interaction time between the microwave and the atom cloud leading to better resolution of the time measurement.

Another way to increase the measurement resolution is to use optical or even ultraviolet transitions in other atomic elements instead of the microwave transition in Cs. This way, one second is not only divided in roughly 10,000,000,000 parts but in up to about 1,000,000,000,000,000 – an improvement in resolution of hundred thousand. In fact, present optical atom clocks based on trapped ions or atoms in optical lattices achieve typical uncertainties of 10-15 to 10-16. At present, the two clocks with highest resolution are based on ion traps of mercury (Hg+) or aluminum (Al+) and achieve uncertainties of 10-17. Such clocks would be wrong by only second in more than 3 billion years! No other measurement can be performed so precisely.  Therefore, the present trend in precision metrology is to convert – if possible – a measurement into a frequency / time measurement.

Fundamental constants and tests of fundamental theories are also performed by frequency metrology, if applicable. The Rydberg constant, for example, is detected by performing high resolution laser spectroscopy of hydrogen and referring the laser frequency to atomic clocks. In order to test the time dependence of the fine structure constant (which should be zero according to presently accepted theory but astronomical observations might indicate that it is not) one can also compare different atom clocks. Other high resolution experiments try measure a non-zero electric dipole moment of the electron, eventually using heavy atoms or molecules. Again, standard model and CPT invariance predict that the EDM should be zero but it is important to test this with higher and higher accuracy. For example, there exist proposed extensions of the standard model that predict deviations from zero at levels that are only two to three orders of magnitude away from present measurement accuracy. So further testing of our understanding of nature is under way. Using very precise and stable clocks of different types, one can also test fundamental principles of special relativity, e.g. isotropy (“Michelson-Morley tests”) or velocity independence (“Kennedy-Thorndike tests”) of speed of light, or even general relativity, e.g. universality of gravitational red shift. These are just a few examples of many interesting experiments, like matter-antimatter comparisons. Atom interferometric determinations of fundamental constants are briefly described below.

Atom interferometry uses wave-like properties of atoms or the atom-light interaction together with the atomic internal states to measure certain quantities in an interferometric way. One detects matter wave interference or a quantum mechanical interference of internal states. An example is a so-called Sagnac interferometer to detect rotations. Using matter waves instead of laser light waves envisages many orders of magnitude higher resolution if the same interferometer area can be realized. Exploiting the photon recoil onto atoms during a (Raman-type) laser excitation, atom interferometry was used to measure the ratio h/m, so the relation between two fundamental quantities with highest accuracy. Combining this result with other precision measurements, also a very accurate value for the hyperfine structure was obtained. An atomic fountain with clouds of free falling atoms can be used to measure the acceleration g due to gravity. The measurement is performed by encoding the vertical position of the atoms in their internal state at three different times with laser induced Raman transitions. The relative number of atoms in one final internal state oscillates between one and zero depending on the phase difference between two possible atomic trajectories within this atom interferometer. Measuring this relative atom number, one can determine the phase difference and extract the value of g so accurately that one can distinguish between different earth tide models. Launching two atom clouds at vertical distance, one can extract also the vertical gradient of g. A further extension to measure the Newtonian gravitational constant G is possible by placing masses close to the atomic trajectories and detecting the influence on the interferometer phase. Similar setups can also be used to measure the gravitational red shift or to detect whether different objects fall in exactly the same way under gravity and hence test the weak equivalence principle. 

Laser-based trace gas analysis makes use of the narrow linewidth of lasers to selectively interact with only one gas or even with just one atomic isotope. Monitoring the absorption or the fluorescence obtained with a laser that is tuned to the proper wavelength one can either detect the density of a gas or monitor its flow. For trace gas analysis with increased isotope selectivity, one can modify the standard IRMS (isotope ratio mass spectroscopy) method which uses segment magnets to separate the paths of different isotopes and then detects their relative occurrence. Instead of a filament based ionization of all isotopes, one uses a narrow linewidth (diode) laser to selectively ionize individual isotopes before they enter the mass filtering element. This way, isotope selectivity up to 1013 was demonstrated. Atom trap trace analysis uses magneto optical traps in order to (isotope-selectively) accumulate also isotopes with very low abundance.     

TOPTICA’s added value 
The high precision measurements that are mentioned here require tunable lasers, most of the time with very narrow linewidth and long term stability. In addition, special electronics modules are needed to perform reliable and most advanced laser stabilization. Photonicals – additional laser related accessories – help to characterize or to manipulate the laser light. Many, if not most experiments mentioned here already successfully use our products. TOPTICA Photonics is proud of its company slogan “A passion for precision.” which since many years describes very well our internal motivation. We are always open for discussions concerning special solutions, are proud to have strong relations to many national institutes or university laboratories and even take part in common research projects related to precision measurements. The pro technology, our latest revolutionary invention, allows us to produce tunable lasers with highest acoustic stability and narrow linewidth that at the same are long term stable and easy to use. The pro series products will allow you to perform the next step in resolution.